Carbon dioxide (CO

2

)

the main gas emitted from fossil burning

is the primary contributor to global warming. Circulating fluidized bed reactor (CFBR) is proved as an energy-efficient method for post-combustion CO

2

capture. The numerical simulation by computational fluid dynamics (CFD) is believed as a promising tool to study CO

2

adsorption process in CFBR. Although three-dimensional (3D) simulations were proved to have better predicting performance with the experimental results

two-dimensional (2D) simulations have been widely reported for qualitative and quantitative studies on gas-solid behavior in CFBR for its higher computational efficiency recently. However

the discrepancies between 2D and 3D simulations have rarely been evaluated by detailed study. Considering that the differences between the 2D and 3D simulations will vary substantially with the changes of independent operating conditions

it is beneficial to lower computational costs to clarify the effects of dimensionality on the numerical CO

2

adsorption runs under various operating conditions. In this work

the comparative analysis for C

O

2

adsorption in 2D and 3D simulations was conducted to enlighten the effects of dimensionality on the hydrodynamics and reaction behaviors

in which the separation rate

species distribution and hydrodynamic characteristics were comparatively studied for both model frames. With both accuracy and computational costs considered

the viable suggestions were provided in selecting appropriate model frame for the studies on optimization of operating conditions

which directly affect the capture and energy efficiencies of cyclic CO

2

capture process in CFBR.