A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin

Jiwei Liu; Yufeng Du; Wuyang Sun; Quanchao Chang; Changsheng Peng

doi:10.1016/j.cjche.2019.12.019

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A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin

Catalysis, Kinetics and Reaction Engineering | Updated：2026-01-06

- A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin
- A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin
- 中国化学工程学报（英文版） 2020年28卷第4期页码：1077-1084
- Affiliations：
  
  1. Key Lab of Marine Environmental Science and Ecology, Ministry of Education, Ocean University of China,Qingdao,China,266100
  2. School of Environment, Tsinghua University,Beijing,China,100084
  3. School of Environmental and Chemical Engineering, Zhaoqing University,Zhaoqing,China,526061
- Author bio：
- Funds：
- DOI：10.1016/j.cjche.2019.12.019
  中图分类号：
- 纸质出版：2020
- Accepted：
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Jiwei Liu, Yufeng Du, Wuyang Sun, 等. A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin[J]. 中国化学工程学报（英文版）, 2020,28(4):1077-1084.

Jiwei Liu, Yufeng Du, Wuyang Sun, Quanchao Chang, Changsheng Peng. A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin[J]. Chinese Journal of Chemical Engineering, 2020, 28(4): 1077-1084.
Jiwei Liu, Yufeng Du, Wuyang Sun, 等. A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin[J]. 中国化学工程学报（英文版）, 2020,28(4):1077-1084. DOI： 10.1016/j.cjche.2019.12.019.

Jiwei Liu, Yufeng Du, Wuyang Sun, Quanchao Chang, Changsheng Peng. A granular adsorbent-supported Fe/Ni nanoparticles activating persulfate system for simultaneous adsorption and degradation of ciprofloxacin[J]. Chinese Journal of Chemical Engineering, 2020, 28(4): 1077-1084. DOI： 10.1016/j.cjche.2019.12.019.

摘要

Abstract

In this work

Fe/Ni nanoparticles were produced through Fe(Ⅱ) and Ni(Ⅱ) reduction by NaBH

and they were stabilized by a kind of prepared granular adsorbent (Fe/Ni@PGA). Fe/Ni@PGA as an environment-friendly activator was used to activate persulfate (PS) for the removal of ciprofloxacin from aqueous solution. Fe/Ni@PGA was systematically characterized via Brunauer-Emmett-Teller (BET) method

X-ray diffraction (XRD)

scanning electron microscopy (SEM)

and Fourier transform infrared spectroscopy (FTIR). The effects of PS concentration

initial solution pH

Fe/Ni@PGA dosage

initial ciprofloxacin concentration

reaction temperature

anions

and natural organic matters on the removal of ciprofloxacin by Fe/Ni@PGA/PS were analyzed. The removal efficiency of ciprofloxacin by Fe/Ni@PGA/PS was 93.24% under an initial pH of 3.0

PS concentration of 10 mM

Fe/Ni@PGA dosage of 0.1 g

and reaction temperature of 30 ℃. Fe/Ni@PGA could still exhibit high catalytic activity after nine cycles of regeneration. The removal mechanisms for ciprofloxacin by the Fe/Ni@PGA/PS system were proposed. In summary

the Fe/Ni@PGA/PS system could be

applied as a promising technology for ciprofloxacin removal.

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