Jianqiu Gao, Chun Li, Weizao Liu, 等. Process simulation and energy integration in the mineral carbonation of blast furnace slag[J]. 中国化学工程学报(英文版), 2019,27(1):157-167.
Jianqiu Gao, Chun Li, Weizao Liu, Jinpeng Hu, Lin Wang, Qiang Liu, Bin Liang, Hairong Yue, Guoquan Zhang, Dongmei Luo, Siyang Tang. Process simulation and energy integration in the mineral carbonation of blast furnace slag[J]. Chin.J.Chem.Eng., 2019, 27(1): 157-167.
Jianqiu Gao, Chun Li, Weizao Liu, 等. Process simulation and energy integration in the mineral carbonation of blast furnace slag[J]. 中国化学工程学报(英文版), 2019,27(1):157-167.DOI: 10.1016/j.cjche.2018.04.012.
Jianqiu Gao, Chun Li, Weizao Liu, Jinpeng Hu, Lin Wang, Qiang Liu, Bin Liang, Hairong Yue, Guoquan Zhang, Dongmei Luo, Siyang Tang. Process simulation and energy integration in the mineral carbonation of blast furnace slag[J]. Chin.J.Chem.Eng., 2019, 27(1): 157-167.DOI: 10.1016/j.cjche.2018.04.012.
Process simulation and energy integration in the mineral carbonation of blast furnace slag
Large quantities of blast furnace (BF) slag and CO
2
are discharged annually from iron and steel industries
along with a large amount of waste heat. The mineral carbonation of BF slag can not only reduce emissions of solid waste but also realize the in-situ fixation of CO
2
with low energy consumption if integrated with the waste heat utilization. In this study
based on our previous works
Aspen Plus was employed to simulate and optimize the carbonation process and integrate the process energy. The effects of gehlenite extraction
MgSO
4
carbonation
and aluminum ammonium sulfate crystallization were studied systematically. The simulation results demonstrate that 2.57 kg of BF slag can sequester 1 kg of CO
2
requiring 5.34 MJ of energy (3.3 MJ heat and 2.04 MJ electricity)
and this energy includes the capture of CO
2
from industrial flue gases. Approximately 60 kg net CO
2
emission reduction could be achieved for the disposal of one ton of BF slag. In addition
the by-product
aluminum ammonium sulfate
is a high value-added product. Preliminary economic analysis indicates that the profit for the whole process i
s 1127 CNY per ton of BF slag processed.
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