Xiaomei Wu, Yunsong Yu, Zhen Qin, 等. Performance of CO2 absorption in a diameter-varying spray tower[J]. 中国化学工程学报(英文版), 2017,25(8):1109-1114. DOI: 10.1016/j.cjche.2017.03.013.
absorption in a diameter-varying spray tower[J]. , 2017, 25(8): 1109-1114.
Xiaomei Wu, Yunsong Yu, Zhen Qin, 等. Performance of CO2 absorption in a diameter-varying spray tower[J]. 中国化学工程学报(英文版), 2017,25(8):1109-1114. DOI: 10.1016/j.cjche.2017.03.013.DOI:
Performance of CO2 absorption in a diameter-varying spray tower
摘要
Abstract
The application of spray towers for CO
2
capture is a development trend in recent years. However
most of the previous jobs were conducted in a cylindrical tower by using a single spray nozzle
whose configuration and performance is not good enough for industrial application. To solve this problem
the present work proposed a diameter-varying spray tower and a new spray mode of dual-nozzle opposed impinging spray to enhance the heat and mass transfer of CO
2
absorption process. Experiments were performed to investigate the mass transfer performance (in terms of the CO
2
removal rate (
η
) and the overall mass transfer coefficient (
K
G
a
e
2 are major factors
which affect the absorption performance and the maximums of
η
and
K
G
a
e
that are 94.0% and 0.574 kmol·m
-3
·h
-1
·kPa
-1
respectively
under the experimental conditions. Furthermore
new correlations to predict the mass transfer coefficient of the proposed spray tower are developed in various CO
2
concentrations with a Pearson Correlation Coefficient over 90%.
关键词
Keywords
references
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