The main purpose of this work was the modification of NaX nanozeolite using copper oxide nanoparticles and various monovalent cations such as K

+

Cs

+

and Ag

+

in order to make the negatively charged zeolite surface accessible for anionic forms of uranium which are the most dominant species of uranium in the contaminated radioactive waters at natural pH. Various methods such as the X-ray fluorescence (XRF)

X-ray powder diffraction (XRD)

field emission scanning electron microscopy (FE-SEM)

transmission electron microscopy (TEM)

Fourier transform infrared spectroscopy (FT-IR)

and atomic absorption spectroscopy (AAS) were used to characterize the final synthesized absorbents. Batch technique was used to study the adsorption behavior of uranium ions from polluted drinking water by NaX nanozeolite and its modified forms. In order to better understand the performance of them

the results were compared with those that were obtained for synthesizing bulk NaX zeolite and Na-form of clinoptilolite natural zeolite. Preliminary results indicated that uranium sorption increased as the loading level of CuO nanoparticles on Na

X nanozeolite increased from 2.1 wt% to 11.2 wt%. In addition

from the obtained data

an increase in uranium removal efficiency resulted as charge/ionic radius ratio of exchanged cation decreased. Also

the effect of contact time

solid-liquid ratio

initial concentration and temperature on the adsorption process was studied. It is worth mentioning that

in this study

the sorption of uranium was performed under natural conditions of pH and the presence of competing cations and anions which are available in drinking waters.