Hadiseh Khalilpourmeymandi, Azadeh Mirvakili, Mohammad Reza Rahimpour, 等. Application of response surface methodology for optimization of purge gas recycling to an industrial reactor for conversion of CO2 to methanol[J]. 中国化学工程学报(英文版), 2017,25(5):676-687. DOI: 10.1016/j.cjche.2016.10.020.
to methanol[J]. , 2017, 25(5): 676-687.
Hadiseh Khalilpourmeymandi, Azadeh Mirvakili, Mohammad Reza Rahimpour, 等. Application of response surface methodology for optimization of purge gas recycling to an industrial reactor for conversion of CO2 to methanol[J]. 中国化学工程学报(英文版), 2017,25(5):676-687. DOI: 10.1016/j.cjche.2016.10.020.DOI:
Application of response surface methodology for optimization of purge gas recycling to an industrial reactor for conversion of CO2 to methanol
摘要
Abstract
Nowadays
by the increasing attention to environment and high rate of fuel production
recycling of purge gas as reactant to a reactor is highly considered. In this study
it is proposed that the purge gases of methanol production unit
which are approximately 15.018 t·h
-1
in the largest methanol production complexes in the world
can be recycled to the reactor and utilized for increasing the production rate. Purge gas streams contain 63% hydrogen
20% carbon monoxide and carbon dioxide as reactants and 17% nitrogen and methane as inert. The recycling effect of beneficial components on methanol production rate has been investigated in this study. Simulation results show that methanol production enhances by recycling just hydrogen
carbon dioxide and carbon monoxide which is an effective configuration among the others. It is named as Desired Recycle Configuration (DRC) in this study. The optimum fraction of returning purge gas is calculated via one dimensional modeling of process and Response Surface Methodology (RSM) is applied to maximize the methanol flow rate and minimize the carbon dioxide flow rat
e. Simulation results illustrate that methanol flow rate increases by 0.106% in DRC compared to Conventional Recycle Configuration (CRC) which therefore shows the superiority of applying DRC to CRC.
关键词
Keywords
references
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相关作者
Zhao Chumeng
Qi Yabing
Yuxin Li
Qunsheng Li
Hongkang Zhao
Zhongwei Ding
Shaolan Zhuang
Xuan Du
相关机构
School of Chemistry and Chemical Engineering, Xi'an University of Architecture and Technology
Inner Mongolia Algal Life Science Co., LTD, Ulanqab
College of Basic Medical Science, Inner Mongolia Medical University, Inner Mongolia Key Lab of Molecular Biology
Engineering Research Center of Preparation Technology of Ultra-Pure Chemicals for Integrated Circuits, Ministry of Education, Beijing University of Chemical Technology
State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology