Process Characteristics of CO2 Absorption by Aqueous Monoethanolamine in a Microchannel Reactor
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Process Characteristics of CO2 Absorption by Aqueous Monoethanolamine in a Microchannel Reactor
Process Characteristics of CO2 Absorption by Aqueous Monoethanolamine in a Microchannel Reactor
中国化学工程学报(英文版)2012年20卷第1期 页码:111-119
Affiliations:
1. Dalian Institute of Chemical Physics, Chinese Academy of Sciences,Dalian,China,116023
2. Graduate School, Chinese Academy of Sciences,Beijing,China,100049
Author bio:
Funds:
Supported by the National Natural Science Foundation of China (20911130358);the Ministry of Science and Technology of China (2009CB219903);the Fund of Dalian Institute of Chemical Physics,CAS (K2009D01)
叶春波, 陈光文, 袁权. Process Characteristics of CO2 Absorption by Aqueous Monoethanolamine in a Microchannel Reactor[J]. 中国化学工程学报(英文版), 2012,20(1):111-119. DOI: 10.1016/S1004-9541(12)60370-X.
Absorption by Aqueous Monoethanolamine in a Microchannel Reactor[J]. , 2012, 20(1): 111-119.
叶春波, 陈光文, 袁权. Process Characteristics of CO2 Absorption by Aqueous Monoethanolamine in a Microchannel Reactor[J]. 中国化学工程学报(英文版), 2012,20(1):111-119. DOI: 10.1016/S1004-9541(12)60370-X.DOI:
Absorption by Aqueous Monoethanolamine in a Microchannel Reactor[J]. , 2012, 20(1): 111-119.DOI: 10.1016/S1004-9541(12)60370-X.
Process Characteristics of CO2 Absorption by Aqueous Monoethanolamine in a Microchannel Reactor
absorption using aqueous monoethanolamine(MEA) in a microchannel reactor were investigated experimentally in this work.A T-type rectangular microchannel with a hydraulic diameter of 408 μm was used.Operating parameters
i.e.temperature
pressure and molar ratio of MEA to CO
2
were studied.Under 3 MPa pressure
the mole fraction of CO
2
in gas phase could decrease from 32.3% to 300×10
-6
at least when gas hourly space velocity ranged from 14400 to 68600 h
-1
and molar ratio of MEA to CO
2
was kept at 2.2.In particular
the effects of temperature on CO
2
absorption flux
mass transfer driving force
gas-liquid contact time and enhancement factor were analyzed in detail and found that mass transfer enhancement by chemical reaction was a crucial factor for the process of CO
2
absorption.
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