Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane
香港科技大学化学与生物分子工程系戈登·麦凯教授退休纪念专刊|Updated:2026-01-06
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Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane
Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane
中国化学工程学报(英文版)2012年20卷第3期 页码:577-588
Affiliations:
Laboratoire de Génie des Procédés Chimiques (LGPC), Université Ferhat Abbas, Sétif, Algérie,19000
Lemnouer Chibane, Brahim Djellouli. Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane[J]. 中国化学工程学报(英文版), 2012,20(3):577-588.
Lemnouer Chibane, Brahim Djellouli. Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane[J]. , 2012, 20(3): 577-588.
Lemnouer Chibane, Brahim Djellouli. Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane[J]. 中国化学工程学报(英文版), 2012,20(3):577-588.DOI: 10.1016/S1004-9541(11)60222-X.
Lemnouer Chibane, Brahim Djellouli. Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane[J]. , 2012, 20(3): 577-588.DOI: 10.1016/S1004-9541(11)60222-X.
Role of Periodic Input Composition and Sweeping Gas for Improvement of Hydrogen Production in a Palladium Membrane Reactor by Partial Oxidation of Methane
The partial oxidation of methane under periodic operation over Ni/γ-Al
2
O
3
catalyst was investigated in a Pd-membrane reactor.The effects of key parameters such as the inlet composition and the sweeping gas on methane conversion and the hydrogen recovery are numerically established with two periodic input functions.In order to analyze the effect of the inputs modulation
the reaction was performed under low steam to methane ratio at a moderate temperature and pressure.It was obtained that to achieve process intensification is to operate the process in a periodic way.The main results show that the periodic input functions can improve the performance of the process compared to the optimal steady state operation.Moreover
there is an optimum amplitude of manipulated inputs leads to a maximum of hydrogen recovery.It is noteworthy that the comparison between the predicted performance
via
the sinusoidal and the square ways show that the better average performance was obtained with the square way.
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