Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method

刘蓓; 王秀林; 唐绪龙; 杨兰英; 孙长宇; 陈光进

doi:10.1016/S1004-9541(11)60057-8

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Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method

Updated：2026-01-06

- Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method
- Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method
- 中国化学工程学报（英文版） 2011年19卷第5期页码：784-791
- Affiliations：
  
  State Key Laboratory of Heavy Oil Processing, China University of Petroleum,Beijing,China,102249
- Author bio：
- Funds：
  
  Supported by the National Natural Science Foundation of China (20925623, 21006126);the Special Funds for Major State Basic Research Program of China (No. 2009CB219504);the Research Funds of China University of Petroleum, Beijing (BJBJRC-2010-01);Beijing Nova Program (2010B069)
- DOI：10.1016/S1004-9541(11)60057-8
  中图分类号：
- 纸质出版：2011
- Accepted：
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刘蓓, 王秀林, 唐绪龙, 等. Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method[J]. 中国化学工程学报（英文版）, 2011,19(5):784-791.

LIU Bei, WANG Xiulin, TANG Xulong, YANG Lanying, SUN Changyu, CHEN Guangjin. Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method[J]. , 2011, 19(5): 784-791.
刘蓓, 王秀林, 唐绪龙, 等. Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method[J]. 中国化学工程学报（英文版）, 2011,19(5):784-791. DOI： 10.1016/S1004-9541(11)60057-8.

LIU Bei, WANG Xiulin, TANG Xulong, YANG Lanying, SUN Changyu, CHEN Guangjin. Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method[J]. , 2011, 19(5): 784-791. DOI： 10.1016/S1004-9541(11)60057-8.

摘要

Abstract

In this work

the absorption-hydration hybrid method was used to recover (hydrogen+nitrogen) from (hydrogen+nitrogen+methane+argon) tail gas mixtures of synthetic ammonia plant through hydrate formation/dissociation. A high-pressure reactor with magnetic stirrer was used to study the separation efficiency. The in-fluences of the concentration of antiagglomerant

temperature

pressure

initial gas-liquid volume ratio

and oil-water volume ratio on the separation efficiency were systematically investigated in the presence of tetrahydro-furan (THF). Antiagglomerant was used to disperse hydrate particles into the condensate phase for water-in-oil emulsion system. Since nitrogen is the material for ammonia production

the objective production in our separation process is (hydrogen+nitrogen). Our experimental results show that by adopting appropriate operating conditions

high concentration of (hydrogen+nitrogen) can be obtained using the proposed technology based on forming hydrate.

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