Adam A. Donaldson, ZHANG Zisheng. Coupled Transport Phenomena in Corrugated Photocatalytic Reactors[J]. 中国化学工程学报(英文版), 2011,19(5):763-772.
Adam A. Donaldson, ZHANG Zisheng. Coupled Transport Phenomena in Corrugated Photocatalytic Reactors[J]. , 2011, 19(5): 763-772.
Adam A. Donaldson, ZHANG Zisheng. Coupled Transport Phenomena in Corrugated Photocatalytic Reactors[J]. 中国化学工程学报(英文版), 2011,19(5):763-772.DOI: 10.1016/S1004-9541(11)60054-2.
Adam A. Donaldson, ZHANG Zisheng. Coupled Transport Phenomena in Corrugated Photocatalytic Reactors[J]. , 2011, 19(5): 763-772.DOI: 10.1016/S1004-9541(11)60054-2.
Coupled Transport Phenomena in Corrugated Photocatalytic Reactors
Corrugated reactors are known for their use in applications requiring UV-exposure
whereby media flowing within the corrugated channel react with a photo-active catalyst impregnated on the surface (i.e. TiO
2
). The performance in these systems is dependent on catalyst properties and reactivity for a given light source
in conjunc-tion with the coupled transport of reactants within the media and photons falling incident to the catalyst surface. Experimental and computational analyses of local mass transfer and radiation patterns for a broad range of corruga-tion angles
depths
and non-idealities introduced during manufacture (i.e. fold curvature) are thus integrated to the design and optimization of these systems. This work explores techniques for determining incident energy distribu-tions on the surface of corrugated reactor geometries with non-ideal cross-sectional profiles
and the local and over-all mass transfer rates obtained using computational fluid dynamics and experimental analysis. By examining the reaction kinetics for the photo-degradation of 4-chlorophenol over a TiO
2
catalyst
the effects of surface area
en-ergy incidence with photon recapture
and local mass transfer on overall reactor performance are presented to high-light optimization concerns for these types of reactors.
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相关作者
Wen-Cong Chen
Ya-Wei Fan
Liang-Liang Zhang
Bao-Chang Sun
Yong Luo
Hai-Kui Zou
Guang-Wen Chu
Jian-feng Chen
相关机构
Research Center of the Ministry of Education for High Gravity Engineering and Technology, Beijing University of Chemical Technology
State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology
School of Chemical Engineering, Sichuan University
State Key Laboratory of Petroleum Molecular & Process Engineering, Institute of Process Engineering, Chinese Academy of Sciences
State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences