Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite
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Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite
Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite
中国化学工程学报(英文版)2022年48卷第8期 页码:66-75
Affiliations:
1. School of Chemical Engineering and Technology, Hebei University of Technology,Tianjin,China,300130
2. University of Rwanda, College of Science and Technology, Kigali,Rwanda,3900
3. Department of Agricultural Microbiology, National Research Centre,Cairo,Egypt,12622
4. College of Mechatronics and Control Engineering, Shenzhen University,Shenzhen,China,518060
Author bio:
Funds:
DOI:
中图分类号:
纸质出版:2022
Accepted:
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Pascal Habimana, Yanjun Jiang, Jing Gao, 等. Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite[J]. 中国化学工程学报(英文版), 2022,48(8):66-75.
Pascal Habimana, Yanjun Jiang, Jing Gao, Jean Bernard Ndayambaje, Osama M. Darwesh, Jean Pierre Mwizerwa, Xiaobing Zheng, Li Ma. Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite[J]. Chinese Journal of Chemical Engineering, 2022, 48(8): 66-75.
Pascal Habimana, Yanjun Jiang, Jing Gao, 等. Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite[J]. 中国化学工程学报(英文版), 2022,48(8):66-75.DOI:
Pascal Habimana, Yanjun Jiang, Jing Gao, Jean Bernard Ndayambaje, Osama M. Darwesh, Jean Pierre Mwizerwa, Xiaobing Zheng, Li Ma. Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite[J]. Chinese Journal of Chemical Engineering, 2022, 48(8): 66-75.DOI:
Enhancing laccase stability and activity for dyes decolorization using ZIF-8@MWCNT nanocomposite
The continuous use of chemical dyes in various industries
and their discharge into industrial effluents
results in severe problems to human life and water pollution. Laccases have the ability to decolorize dyes and toxic chemicals in industrial effluents as green biocatalysts. Their possible industrial applications have been limited by poor reusability
low stability
and loss of free laccase action. In this research
laccase was immobilized on zeolitic imidazolate framework coated multi-walled carbon nanotubes (Laccase@ZIF-8@MWCNTs)
via
metal affinity adsorption to develop an easy separable and stable enzyme. The optimum reaction conditions for immobilized laccase are at a pH of 3.0 and a temperature of 60?℃. The immobilized laccase was enhanced in storage and thermal stability. The results indicated that Laccase@ZIF-8@MWCNTs still maintained 68% of its original activity after 10 times of repeated use. Most importantly
the biocatalytic system was applied for decolorization of different dyes (20?mg·L
?1
) without a mediator
and up to 97.4% for Eriochrome black T and 95.6% Acid red 88 was achieved in 25 min. Biocatalysts with these properties may be used in a variety of environmental and industrial applications.
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相关作者
Yi Liu
Fei Wang
Taotao Ji
Yuyang Wu
Xinmiao Jin
Sixing Chen
Xuke Zhang
Yafei Su
相关机构
Dalian Key Laboratory of Membrane Materials and Membrane Processes, Dalian University of Technology
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences
State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials, School of Chemical Engineering, Dalian University of Technology
School of Material & Chemical Engineering, Zhengzhou University of Light Industry
Research Department of New Materials, Zhengzhou Institute of Emerging Industrial Technology