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1. State Key Laboratory of Heavy Oil Processing, China University of Petroleum,Beijing,China,102249
2. School of Chemistry and Chemical Engineering, Changsha University of Science & Technology,Changsha,China,410114
Published:2024
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storage in hydrate-bearing sediments
DOI:
storage in hydrate-bearing sediments DOI: 10.1016/j.cjche.2023.09.016.
Carbon emission reduction and clean energy development are urgent demands for mankind in the coming decades. Exploring an efficient CO
2
storage method can significantly reduce CO
emissions in the short term. In this study
we attempted to construct sediment samples with different residual CH
4
hydrate amounts and reservoir conditions
and then investigate the potentials of both CO
storage and enhanced CH
recovery in depleted gas hydrate deposits in the permafrost and ocean zones
respectively. The results demonstrate that CO
hydrate formation rate can be significantly improved due to the presence of residual hydrate seeds; However
excessive residual hydrates in turn lead to the decrease in CO
storage efficiency. Affected by the
T-P
conditions of the reservoir
the storage amount of liquid CO
can reach 8 times that of gaseous CO
and CO
stored in hydrate form reaches 2-4 times. Additionally
we noticed two other advantages of this method. One is that CO
injection can enhance CH
recovery rate and increases CH
recovery by 10%-20%. The second is that hydrate saturation in the reservoir can be restored to 20%-40%
which means that the solid volume of the reservoir avoids serious shrinkage. Obviously
this is crucial for protecting the goaf stability. In summary
this approach is great
ly promising for high-efficient CO
storage and safe exploitation of gas hydrate.
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