Recent advances in non-thermal plasma (NTP) catalysis towards C1 chemistry

Huanhao Chen; Yibing Mu; Shanshan Xu; Shaojun Xu; Christopher Hardacre; Xiaolei Fan

doi:10.1016/j.cjche.2020.05.027

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Recent advances in non-thermal plasma (NTP) catalysis towards C1 chemistry

Reviews | Updated：2026-01-06

- Recent advances in non-thermal plasma (NTP) catalysis towards C1 chemistry
- Chinese Journal of Chemical Engineering Vol. 28, Issue 8, Pages: 2010-2021(2020)
- Affiliations：
  
  1. State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University,Nanjing,China,210009
  2. Department of Chemical Engineering and Analytical Science, School of Engineering, The University of Manchester, M13 9PL, United Kingdom
  3. School of Chemistry, Cardiff University, Main Building, Park Place, Cardiff CF10 3AT, United Kingdom
  4. UK Catalysis Hub, Research Complex at Harwell, Rutherford Appleton Laboratory, Harwell, Oxon OX11 0FA, United Kingdom
- Author bio：
- Funds：
- DOI：10.1016/j.cjche.2020.05.027
  CLC：
- Published：2020
- Accepted：
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Huanhao Chen, Yibing Mu, Shanshan Xu, Shaojun Xu, Christopher Hardacre, Xiaolei Fan. Recent advances in non-thermal plasma (NTP) catalysis towards C1 chemistry[J]. Chinese Journal of Chemical Engineering, 2020, 28(8): 2010-2021.
DOI：

Huanhao Chen, Yibing Mu, Shanshan Xu, Shaojun Xu, Christopher Hardacre, Xiaolei Fan. Recent advances in non-thermal plasma (NTP) catalysis towards C1 chemistry[J]. Chinese Journal of Chemical Engineering, 2020, 28(8): 2010-2021. DOI： 10.1016/j.cjche.2020.05.027.

摘要

Abstract

C1 chemistry mainly involves the catalytic transformation of C1 molecules (

i.e

and CH

OH)

which usually encounters thermodynamic and/or kinetic limitations. To address these limitations

non-thermal plasma (NTP) activated heterogeneous catalysis offers a number of advantages

such as relatively mild reaction conditions and energy efficiency

in comparison to the conventional thermal catalysis. This review presents the state-of-the-art for the application of NTP-catalysis towards C1 chemistry

including the CO

hydrogenation

reforming of CH

and CH

and water-gas shift (WGS) reaction. In the hybrid NTP-catalyst system

the plasma-catalyst interactions are multifaceted. Accordingly

this review also includes a brief discussion on the fundamental research into the mechanisms of NTP activated catalytic C1 chemistry

such as the advanced characterisation methods (

e.g

in situ

diffuse reflectance infrared Fourier transform spectroscopy

DRIFTS)

temperatureprogrammed plasma surface reaction (TPPSR)

kinetic studies. Finally

prospects for the future research on the development of tailor-made catalysts for NTP-catalysis systems (which will enable the further understan

ding of its mechanism) and the translation of the hybrid technique to practical applications of catalytic C1 chemistry are discussed.

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