Systematic investigation of SO2 adsorption and desorption by porous powdered activated coke: Interaction between adsorption temperature and desorption energy consumption
|Updated:2026-01-06
|
Systematic investigation of SO2 adsorption and desorption by porous powdered activated coke: Interaction between adsorption temperature and desorption energy consumption
Chinese Journal of Chemical EngineeringVol. 48, Issue 8, Pages: 140-148(2022)
Affiliations:
1. National Engineering Laboratory for Reducing Emissions from Coal Combustion, Engineering Research Center of Environmental Thermal Technology of Ministry of Education, Shandong Key Laboratory of Energy Carbon Reduction and Resource Utilization, School of Energy and Power Engineering, Shandong University,Jinan,China,250061
2. College of Mechanical and Electronic Engineering, Shandong University of Science and Technology,Qingdao,China,266590
Author bio:
Funds:
DOI:
CLC:
Published:2022
Accepted:
Scan QR Code
adsorption and desorption by porous powdered activated coke: Interaction between adsorption temperature and desorption energy consumption[J]. 中国化学工程学报, 2022, 48(8): 140-148.
DOI:
adsorption and desorption by porous powdered activated coke: Interaction between adsorption temperature and desorption energy consumption[J]. 中国化学工程学报, 2022, 48(8): 140-148.DOI:
Systematic investigation of SO2 adsorption and desorption by porous powdered activated coke: Interaction between adsorption temperature and desorption energy consumption
Porous carbon materials have been widely used for the removal of SO
2
from flue gas. The main objective of this work is to clarify the effects of adsorption temperature on SO
2
adsorption and desorption energy consumption. Coal-based porous powdered activated coke (PPAC) prepared in the drop-tube reactor was used in this study. The N
2
adsorption measurements and Fourier transform infrared spectrometer analysis show that PPAC exhibits a developed pore structure and rich functional groups. The experimental results show that with a decrease in adsorption temperature in the range of 50–150?℃
the adsorption capacity of SO
2
increases linearly; meanwhile
the adsorption capacity of H
2
O increases
resulting in the increase in desorption energy consumption per unit mass of adsorbent. The processes of SO
2
and H
2
O desorption were determined by the temperature-programmed desorption test
and the desorption energies for each species were calculated. Considering the energy consumption per unit of desorption and the total amount of adsorbent
the optimal adsorption temperature yielding the minimum total energy consumption of regeneration is calculated. This study systematically demonstrates the effect of adsorption temperature on the adsorption–desorption process
providing a basis for energy saving and emission reduction in desulfurization sys
tem design.
关键词
Keywords
references
The trial reading is over, you can activate your VIP account to continue reading.
Study of the reaction mechanism for preparing powdered activated coke with SO2 adsorption capability via one-step rapid activation method under flue gas atmosphere
Nano-confinement construction of FeCo@NCNTs nanocomposite for pH-universal oxygen reduction catalysis and high-power Zn-air battery
Dynamic behavior of a single bubble in cavity flow driven by a turbulent channel
Optimizing energy efficiency in fluid catalytic cracking units with GA and NSGA-II: A comprehensive simulation and multi-factor analysis
Synthesis of chemiluminescent carbonized polymer dots under atmospheric conditions for multimode luminescence anti-counterfeiting
Related Author
Binxuan Zhou
Jingcai Chang
Jun Li
Jinglan Hong
Tao Wang
Liqiang Zhang
Ping Zhou
Chunyuan Ma
Related Institution
School of Environmental Science and Engineering, Shandong University
Weihai Research Institute of Industrial Technology of Shandong University
School of Energy and Power Engineering, Shandong University