Accurately predicting distributions of concentration and temperature field in fixed-bed column is essential for designing adsorption processes. In this study
a two-dimensional (2D)
axisymmetric
nonisothermal
dynamic adsorption model was established by coupling equations of mass
momentum and energy balance
and solved by finite element analysis. The simulation breakthrough curves fit well with the low-concentration CO
2
adsorption experimental data
indicating the reliability of the established model. The distributions of concentration and temperature field in the column for CO
2
adsorption and separation from CO
2
/N
2
were obtained. The sensitivity analysis of the adsorption conditions shows that the operation parameters such as feed flow rate
feed concentration
pellet size
and column height-to-diameter ratio produce a significant effect on the dynamic adsorption performance. The multi-physics coupled 2D axisymmetric model could provide a theoretical foundation and guidance for designing CO
2
fixed-bed adsorption and separation processes
which could be extended to other mixed gases as well.
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Parametric study and effect of calcination and carbonation conditions on the CO2 capture performance of lithium orthosilicate sorbent
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